منابع مشابه
Biphasic water splitting by osmocene.
The photochemical reactivity of osmocene in a biphasic water-organic solvent system has been investigated to probe its water splitting properties. The photoreduction of aqueous protons to hydrogen under anaerobic conditions induced by osmocene dissolved in 1,2-dichloroethane and the subsequent water splitting by the osmocenium metal-metal dimer formed during H(2) production were studied by elec...
متن کاملMicroscale pH regulation by splitting water.
We present a simple, flexible approach for pH regulation in micro-chambers by injecting controllable amounts of protons and hydroxide ions via field-enhanced dissociation of water molecules. Under a DC voltage bias, the polymeric bipolar membranes integrated in microfluidics devices generate and separate H(+) and OH(-) ions without gas production or contaminant generation resulting from electro...
متن کاملThermochemical water splitting cycles
Two processes to effect splitting of the water molecule by means of an external heat source are competing for adoption, for the long-term production of hydrogen: high-temperature electrolysis, and splitting the water molecule through a succession of chemical reactions: a thermochemical cycle. Both processes form part of a strategy of voluntary reduction of greenhouse-gas emissions, and of alter...
متن کاملSolar water splitting cells.
Energy harvested directly from sunlight offers a desirable approach toward fulfilling, with minimal environmental impact, the need for clean energy. Solar energy is a decentralized and inexhaustible natural resource, with the magnitude of the available solar power striking the earth’s surface at any one instant equal to 130 million 500 MW power plants.1 However, several important goals need to ...
متن کاملPhotoinduced water splitting in pyridine water clusters.
Ab initio calculations predict that pyridine (Py) can act as a photo-catalyst to split water by the absorption of a UV photon following the reaction Py-H2O + hν → PyH˙ + OH˙. To test this prediction, we performed two types of experiments: in the first, we characterize the electronic spectroscopy of the PyH˙ radical in the gas phase. In the second, we evidence the reaction through the UV excitat...
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ژورنال
عنوان ژورنال: Nature Energy
سال: 2020
ISSN: 2058-7546
DOI: 10.1038/s41560-020-00726-0